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FLOATSUBSCRIPTCl under 115 K. Its Br-containing analogue is stable in the room-temperature crystal structure right down to at the very least 10 Ok, although the Br compound is on the verge of a similar antiferroelectric instability and reveals local displacements of Cu and Br atoms. The I-containing compound is stable in its room-temperature structure in response to density-useful calculations. These parameters are chosen in a semi-empirical method as offering greatest settlement with the experimental exchange couplings in previous DFT calculations for francisites Rousochatzakis et al. Quick-range AFM order is formed round 50 K, however no signatures of long-vary ordering are seen down to 2 Ok. This habits may be rationalized on the microscopic degree by the spin lattice comprising sturdy non-annoyed one-dimensional (1D) units with only weak and annoyed couplings between them. FLOATSUBSCRIPTCl, but its magnetic habits is remarkably different. This habits is rationalized microscopically in terms of a non-pissed off 1D spin ladder (tube) with comparatively weak and annoyed couplings between the 1D items. ARG antiferromagnets could be orders of magnitude lower than the energy scale of exchange couplings Janson et al. FLOATSUBSCRIPT tetrahedra. Many of the exchange couplings happen between nearest neighbors, but dissimilar interactions on the edges of those tetrahedra largely scale back the frustration and render the spin lattice quasi-1D.
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